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Nonequilibrium GW+EDMFT: Antiscreening and inverted populations from nonlocal correlations
Department of Physics, University of Fribourg, Fribourg, Switzerland.
Department of Physics, University of Fribourg, Fribourg, Switzerland.
Department of Physics, University of Fribourg, Fribourg, Switzerland.ORCID-id: 0000-0002-7263-4403
Max-Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany.
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2017 (engelsk)Inngår i: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 118, nr 24, artikkel-id 246402Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

We study the dynamics of screening in photo-doped Mott insulators with long-ranged interactions using a nonequilibrium implementation of the GW plus extended dynamical mean field theory (GW+EDMFT) formalism. Our study demonstrates that the complex interplay of the injected carriers with bosonic degrees of freedom (charge fluctuations) can result in long-lived transient states with properties that are distinctly different from those of thermal equilibrium states. Systems with strong nonlocal interactions are found to exhibit a self-sustained population inversion of the doublons and holes. This population inversion leads to low-energy antiscreening which can be detected in time-resolved electron-energy loss spectra. 

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American Physical Society , 2017. Vol. 118, nr 24, artikkel-id 246402
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URN: urn:nbn:se:oru:diva-89905DOI: 10.1103/PhysRevLett.118.246402ISI: 000403341900007Scopus ID: 2-s2.0-85020509581OAI: oai:DiVA.org:oru-89905DiVA, id: diva2:1531082
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Funding Agencies:

European Research Council (ERC)

European Commission 278023

European Research Council (ERC)

European Commission 724103

Swiss National Science Foundation through NCCR MARVEL 200021-165539

German Research Foundation (DFG) 925B4

Tilgjengelig fra: 2021-02-25 Laget: 2021-02-25 Sist oppdatert: 2021-02-26bibliografisk kontrollert

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