Nonequilibrium GW+EDMFT: Antiscreening and inverted populations from nonlocal correlationsShow others and affiliations
2017 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 118, no 24, article id 246402Article in journal (Refereed) Published
Abstract [en]
We study the dynamics of screening in photo-doped Mott insulators with long-ranged interactions using a nonequilibrium implementation of the GW plus extended dynamical mean field theory (GW+EDMFT) formalism. Our study demonstrates that the complex interplay of the injected carriers with bosonic degrees of freedom (charge fluctuations) can result in long-lived transient states with properties that are distinctly different from those of thermal equilibrium states. Systems with strong nonlocal interactions are found to exhibit a self-sustained population inversion of the doublons and holes. This population inversion leads to low-energy antiscreening which can be detected in time-resolved electron-energy loss spectra.
Place, publisher, year, edition, pages
American Physical Society , 2017. Vol. 118, no 24, article id 246402
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:oru:diva-89905DOI: 10.1103/PhysRevLett.118.246402ISI: 000403341900007Scopus ID: 2-s2.0-85020509581OAI: oai:DiVA.org:oru-89905DiVA, id: diva2:1531082
Note
Funding Agencies:
European Research Council (ERC)
European Commission 278023
European Research Council (ERC)
European Commission 724103
Swiss National Science Foundation through NCCR MARVEL 200021-165539
German Research Foundation (DFG) 925B4
2021-02-252021-02-252021-02-26Bibliographically approved